Collective properties of Pb-206, Pb-207, Pb-208 and Bi-209 have been inves
tigated With gamma-ray spectroscopy using electromagnetic excitation by Pb-
208 projectiles. By measuring the absolute yields of the de-excitation gamm
a-rays, B(E3) values for the 1-phonon octupole vibrational states were obta
ined. While the present data for Pb-208 and 209Bi are consistent with earli
er publications, much smaller values have been found for Pb-206 and Pb-207.
Only for the doubly magic nucleus Pb-208 One observes the largest octupole
collectivity of 34 Weisskopf units (W.u.), which is reduced to 60-70% by t
he particle-vibration coupling in nuclei which consist of the Pb-208 core p
lus (or minus) a few nucleons. As a consequence of the phonon vibration cha
racter of the 3(-) state, one expects a quadruplet of 2-phonon octupole sta
tes with spins and parities 0(+), 2(+), 4(+) and 6(+) at about twice the en
ergy of the 1-phonon state, i.e. around 5.23 MeV. A first seat; tering expe
riment suggesting the observation of at least one member of the 2-phonon mu
ltiplet was performed via the reaction Pb-208+Pb-208 at an incident energy
well above the Coulomb barrier In the present experiment the system Pb-208Pb-208 has been reinvestigated via Coulomb excitation at a safe bombarding
energy of 5.0 MeV/u. The reduced cross-section for the excitation of the oc
tupole states has been compensated by the higher full energy efficiency of
five EUROBALL CLUSTER detectors. With the present experimental set-up trans
ition probabilities down to 10(-5)-10(-6) can be measured.